ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Determining the ground state and dynamics in herbertsmithite single crystals: a spinon-mediated liquid state?

Abstract: Previous local-probe experiments have established herbertsmithite, a material containing kagome layers of Cu2+ spins, as one of the most important model systems for exploring quantum spin-liquid (QSL) behaviour. Herbertsmithite realizes a QSL ground state whose precise nature, whether gapped or gapless, has remained under active debate. A recent breakthrough study revealed a pronounced peak in the magnetic susceptibility and spin noise around ~ 260 mK. This has been interpreted as a glassy state that results from spinon interactions mediated by the presence of a gapped Z2 spin-liquid state. Since single-crystal and powder samples of kagome systems can give distinct magnetic responses, and because an earlier muSR measurement was performed on powder specimens, it is now vital to re-examine the low-temperature magnetic behavior of single-crystal herbertsmithite using muSR. We intend to perform zero-field (ZF) and longitudinal-field (LF) muSR measurements to probe the presence or absence, and nature, of any magnetic ordering or the formation of a glassy state, and to characterize the low-energy spin dynamics.

Principal Investigator: Dr Dipranjan Chatterjee
Experimenter: Mr Ewan Thomas
Local Contact: Dr Francis Pratt
Experimenter: Professor Stephen Blundell
Experimenter: Dr Benjamin Huddart
Experimenter: Dr Hank C H Wu

DOI: 10.5286/ISIS.E.RB2610535

ISIS Experiment Number: RB2610535

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB2610535-1 HIFI 03 June 2029 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Dr Dipranjan Chatterjee et al; (2026): Determining the ground state and dynamics in herbertsmithite single crystals: a spinon-mediated liquid state?, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2610535

Data is released under the CC-BY-4.0 license.



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