ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Determining the Magnetic Structure of a Spin-1 Kitaev Candidate Material

Abstract: A family of 2D honeycomb magnets, Na?Ni?XO? (X = Sb, Bi), has garnered interest as a platform for realizing higher-spin Kitaev interactions. In Na?Ni?BiO? (NNBO), a 1/3 magnetization plateau?indicative of bond-dependent Kitaev exchange?has recently been observed, highlighting the potential of this material class to host spin-1 Kitaev physics. We propose neutron powder diffraction on Na?Ni?SbO? (NNSO), the Sb analogue of NNBO, to determine its zero-field magnetic structure. NNSO offers a unique opportunity to probe the influence of anion spin-orbit coupling on Kitaev interactions. Our single-crystal neutron data reveal a propagation vector distinct from that of NNBO, suggesting a different magnetic ground state. The proposed measurements will provide critical structural insight and inform theoretical modeling of spin-1 Kitaev systems.

Principal Investigator: Dr Yanyan Shangguan
Experimenter: Professor Jinsheng Wen
Local Contact: Dr Pascal Manuel
Experimenter: Dr Song Bao

DOI: 10.5286/ISIS.E.RB2520129

ISIS Experiment Number: RB2520129

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB2520129-1 WISH 30 November 2028 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Dr Yanyan Shangguan et al; (2025): Determining the Magnetic Structure of a Spin-1 Kitaev Candidate Material, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2520129

Data is released under the CC-BY-4.0 license.



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