ISIS Neutron and Muon Source Data Journal
This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.
Structural insight into hydrogen adsorption mechanism in a Zr-based MOF using neutron powder diffraction
Abstract: Hydrogen gas (H?) plays an increasingly crucial role in the global transition toward sustainable energy, serving as a clean, efficient, and versatile energy carrier. When used as fuel, hydrogen produces only water as a byproduct. This makes hydrogen an attractive option for powering vehicles, generating electricity, and providing heat, all without carbon emissions. Metal-organic frameworks (MOFs), composed of metal ions or clusters connected by organic linkers, have demonstrated great promise in advancing H2 storage technology. Several MOFs with high gravimetric hydrogen storage capacities have been discovered, such as MOF-177 (11 wt.%, 77K, 70 bar) and NU-100 (16.4 wt.%, 77k, 70 bar). However, as research progressed, our group and others began to recognise the comparative importance of volumetric capacity, and it became clear that a trade-off exists between volumetric and gravimetric H2 storage. Various strategies have been developed to address this challenge, including densifying MOFs into monolithic forms and designing new high-density MOFs
Principal Investigator: Dr David Fairen-Jimenez
Experimenter: Mr Mohammad Reza Alizadeh Kiapi
Local Contact: Dr Pascal Manuel
Experimenter: Dr X Chen
Experimenter: Dr Lik Hong Wee
Experimenter: Mr Hamish William MacLeod
DOI: 10.5286/ISIS.E.RB2520094
ISIS Experiment Number: RB2520094
| Part DOI | Instrument | Public release date | Download Link |
|---|---|---|---|
| 10.5286/ISIS.E.RB2520094-1 | WISH | 06 December 2028 | Download |
Publisher: STFC ISIS Neutron and Muon Source
Data format: RAW/Nexus
Select the data format above to find
out more about it.
Data Citation
The recommended format for citing this dataset in a research
publication is as:
[author], [date], [title], [publisher],
[doi]
For Example:
Dr David Fairen-Jimenez et al; (2025): Structural insight into hydrogen adsorption mechanism in a Zr-based MOF using neutron powder diffraction, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2520094
Data is released under the CC-BY-4.0 license.
