ISIS Neutron and Muon Source Data Journal
This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.
Effect of hydrothermal aging on the proton distribution in Cu-CHA zeolite catalysts
Abstract: Cu-CHA zeolites are excellent catalysts for the removal of NOx from diesel vehicle exhaust gases, through the NH3-SCR reaction. Even if they are outperforming other Cu-zeolites for their activity and hydrothermal stability, the harsh conditions of temperature and presence of water vapour in the exhaust can cause the phenomenon called dealumination, which removes Al atoms from the framework and causes deactivation. We want to study the effect of hydrothermal ageing on the distribution of OH groups in Cu-CHA by means of Inelastic Neutron Scattering on the high resolution instrument TOSCA, to understand the main parameters affecting stability.
Principal Investigator: Professor Gloria Berlier
Experimenter: Dr Anna Marsicano
Experimenter: Dr Ton Victor Willibrord Janssens
Experimenter: Mr Vasco António Correia Saltão
Experimenter: Ms Shivangi Singh
Local Contact: Dr Jeff Armstrong
Experimenter: Mr Gionata Galliano
DOI: 10.5286/ISIS.E.RB2510703
ISIS Experiment Number: RB2510703
| Part DOI | Instrument | Public release date | Download Link |
|---|---|---|---|
| 10.5286/ISIS.E.RB2510703-1 | TOSCA | 12 May 2028 | Download |
Publisher: STFC ISIS Neutron and Muon Source
Data format: RAW/Nexus
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Data Citation
The recommended format for citing this dataset in a research
publication is as:
[author], [date], [title], [publisher],
[doi]
For Example:
Professor Gloria Berlier et al; (2025): Effect of hydrothermal aging on the proton distribution in Cu-CHA zeolite catalysts, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2510703
Data is released under the CC-BY-4.0 license.
