ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Inelastic Neutron scattering study of Crystal Field Effect in CeAgAl3 and PrAgAl3

Abstract: Kondo lattice systems CeCuAl3 and Ag-doped CeCu1-xAgxAl3 (x ? 0.3) present clear evidence for rare phenomenon of magnetoelastic coupling of crystal electric field (CEF) excitations and lattice vibrons. This motivated us to investigate the spin dynamics and CEF excitations in the end point compound CeAgAl3 which should help us understand the origin of magnetoelastic coupling in CeCu1-xAgxAl3 (0 ? x ? 0.3). CeAgAl3 forms in orthorhombic Cmcm structure which admits Ag/Al site-mixing. It has ferromagnetically ordered ground state below 3.8 K, but the short range magnetic correlations develop below 15 K. PrAgAl3 which also forms in orthorhombic Cmcm structure orders ferromagnetically below 5.5 K. We performed MERLIN express measurements on CeAgAl3 [RB2490017] and obtained interesting CEF excitations, but statistics is not enough for the publication. Further investigations of RAgAl3 (R=Ce and Pr) using the inelastic neutron scattering experiment are highly desired to determine the crystal field states of these compounds in order to understand the effect of single ion anisotropy. We propose to carry inelastic neutron scattering measurements on CeAgAl3 and PrAgAl3 using MARI spectrometer to determine the crystal field level scheme.

Principal Investigator: Dr Vivek Kumar Anand
Local Contact: Dr Duc Le
Experimenter: Dr Devashi Adroja
Experimenter: Dr Uthayakumar Sivaperumal

DOI: 10.5286/ISIS.E.RB2510185

ISIS Experiment Number: RB2510185

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB2510185-1 MARI 22 April 2028 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Dr Vivek Kumar Anand et al; (2025): Inelastic Neutron scattering study of Crystal Field Effect in CeAgAl3 and PrAgAl3, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2510185

Data is released under the CC-BY-4.0 license.



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