ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Characterization of ionic liquid dynamics within composite graphene-ionic liquid supercapacitor electrodes

Abstract: Supercapacitors are a promising renewable alternative to devices for mobile power supply. Rapid energy storage is achieved via the formation of a double-layer of electronic and ionic charge at the electrode/electrolyte interface. Active material pore structure/surface area and distribution of ions that bind to the electrode surface are key performance indicators. Commercially used activated carbons demonstrate adequate gravimetric energy density, Eg, but low density leads to poor volumetric energy density, Ev. Graphene is an ideal candidate, whilst reduced graphene oxide exhibits greater capacitance. Electrode pore utilization can be increased by greater electrolyte pore integration whilst energy density can be increased by use of large electrochemical voltage window electrolytes. Ionic liquids (IL) have thus become promising next-generation electrolytes. Here we will study the dynamics of IL confined within the intralayer voids; these together with our previous structural characterisation will provide further insight to the charging mechanism within this novel electrode system and aid our understanding of the structure-property relationships at different compositions.

Principal Investigator: Professor Michael Pope
Experimenter: Dr Ross Stewart
Experimenter: Dr Keenan Smith
Experimenter: Dr Andrew Seel
Experimenter: Dr Fabrizia Foglia
Experimenter: Dr Victoria Garcia Sakai
Local Contact: Dr Gøran Nilsen
Experimenter: Mr Tianyu Liu
Experimenter: Mr Adam Morris
Local Contact: Dr Mona Sarter

DOI: 10.5286/ISIS.E.RB2467013

ISIS Experiment Number: RB2467013

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB2467013-1 LET 31 July 2027 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Professor Michael Pope et al; (2026): Characterization of ionic liquid dynamics within composite graphene-ionic liquid supercapacitor electrodes, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2467013

Data is released under the CC-BY-4.0 license.



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