ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Magnetic Properties of Molecular p-d System l-(BEDT-STF)2FexGa1-xCl4

Abstract: The purpose of this proposal is to reveal the mechanism of the peculiar magnetism observed in molecular p-d system l-(BEDT-STF)2FexGa1-xCl4, where BEDT-STF is bis(ethylenedithio)diselenadithiafulvalene. l-(BEDT-STF)2FexGa1-xCl4 shows a peculiar magnetic property that the local fields at Fe sites show a step-like development below an antiferromagnetic transition temperature (TN). The mechanism of the peculiar magnetism is considered to be derived from the magnetic coupling between p electrons with strong electron correlation and localized 3d spins. In this proposal, we investigate the Fe concentration dependence of the TN and the local fields at Fe sites. By controlling the Fe concentration, we can modulate the strength of the magnetic coupling systematically. From the results, we discuss the relationship between the coupling effect and the mechanism of the peculiar magnetism.

Principal Investigator: Dr Shuhei Fukuoka
Local Contact: Dr Isao Watanabe
Experimenter: Professor Atsushi KAWAMOTO

DOI: 10.5286/ISIS.E.RB1970118

ISIS Experiment Number: RB1970118

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB1970118-1 HIFI 12 June 2024 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Dr Shuhei Fukuoka et al; (2021): Magnetic Properties of Molecular p-d System l-(BEDT-STF)2FexGa1-xCl4, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB1970118

Data is released under the CC-BY-4.0 license.



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