ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Investigation of Vibronic Excitations in Ce2O3

Abstract: Hybrid modes are often associated with quantum ground states and other novel emergent phenomena. One such hybrid mode, the vibronic mode, is a bound state between a crystal electric field (CEF) and a phonon. These modes, long predicted in systems where lattice vibrations significantly alter the CEF strength at a large moment spin site, are expected to precipitate unique spin-lattice coupling mechanisms. A recent Raman spectroscopy study revealed the emergence of two new modes below a purported antiferromagnetic transition at T=6.2K. These new modes were identified as vibronic excitations, though a thorough investigation of the CEF and phonon spectrum is required to strengthen this claim. For this reason, we seek to use MERLIN to map the evolution of CEF and phonon modes in Ce2O3 at temperatures both above and below the antiferromagnetic transition.

Principal Investigator: Professor Gregory MacDougall
Experimenter: Ms Alexandra Cote
Local Contact: Dr Devashi Adroja

DOI: 10.5286/ISIS.E.RB2000208

ISIS Experiment Number: RB2000208

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.RB2000208-1 MERLIN 31 May 2024 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Professor Gregory MacDougall et al; (2021): Investigation of Vibronic Excitations in Ce2O3, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB2000208

Data is released under the CC-BY-4.0 license.



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