ISIS Neutron and Muon Source Data Journal

In Operando Diffusion Measurements on an All Solid-State Garnet Battery Cell by Muon Spin Relaxation Spectroscopy

Abstract: The development of all-solid state batteries is of significant interest as a solid electrolyte enables the removal of the flammable solvent phase and is stable to much higher potentials than modern batteries. We wish to perform in situ measurements on two all solid-state batteries to develop our fundamental understanding of the diffusion processes that occur during cycling. The all solid-state garnet materials under investigation offer excellent structural stability, high ionic conductivities, and do not react in contact with lithium metal anode. By studying the interfacial diffusion with a structurally equivalent electrode we hope to greatly enhance our understanding of the lithium diffusion mechanisms and rates, enabling further structural modifications to enhance the beneficial properties within a future all solid-state battery.

Principal Investigator: Professor Serena Cussen
Experimenter: Dr Sam Booth
Experimenter: Dr Beth Johnston
Local Contact: Dr Peter Baker
Experimenter: Dr Innes McClelland
Experimenter: Dr Hany ElShinawi
Experimenter: Professor Edmund Cussen
Experimenter: Miss Jasmin Clough

DOI: 10.5286/ISIS.E.RB1920550

ISIS Experiment Number: RB1920550

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Professor Serena Cussen et al; (2019): In Operando Diffusion Measurements on an All Solid-State Garnet Battery Cell by Muon Spin Relaxation Spectroscopy, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB1920550

Data is released under the CC-BY-4.0 license.