ISIS Neutron and Muon Source Data Journal

This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.


Uranium minerals related to geochemical storage of spent nuclear fuels: a powder neutron diffraction study

Abstract: The safe storage of spent nuclear fuels is a complex challenge that belies a simple solution. The biggest scientific challenge is that storage must be over long periods of time, and knowledge of how the complex and interlinked chemistry changes is important to build robust safety cases for underground storage. One important uranium compound is studtite, [UO2(O2)(H2O)2].2H2O which dehydrates to metastudtite [UO2(O2)(H2O)2]. There are subtle structural changes that may impact on the chemical behaviour. In this project we aim to look at the dehydration using powder neutron diffraction to precisely locate the light atoms (oxygen and hydrogen) and explore these structural effects.

Principal Investigator: Dr Robert Baker
Experimenter: Mr Samuel Edwards
Local Contact: Dr Dominic Fortes

DOI: 10.5286/ISIS.E.RB1820012

ISIS Experiment Number: RB1820012

Part DOI Instrument Public release date Download Link
10.5286/ISIS.E.98020062 HRPD 26 September 2021 Download
10.5286/ISIS.E.RB1820012-2 HRPD 08 December 2022 Download
10.5286/ISIS.E.RB1820012-3 HRPD 14 March 2023 Download
10.5286/ISIS.E.RB1820012-4 HRPD 18 May 2024 Download
10.5286/ISIS.E.RB1820012-5 HRPD 23 May 2024 Download

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
Select the data format above to find out more about it.

Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Dr Robert Baker et al; (2018): Uranium minerals related to geochemical storage of spent nuclear fuels: a powder neutron diffraction study, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB1820012

Data is released under the CC-BY-4.0 license.



UKRI


Science and Technology Facilities Council Switchboard: 01793 442000