This is a page describing data taken during an experiment at the ISIS Neutron and Muon Source. Information about the ISIS Neutron and Muon Source can be found at https://www.isis.stfc.ac.uk.
Studies of catalyst-substrate interactions in an industrial ZSM-5 cracking catalyst
Abstract: ZSM-5 zeolites are used as additives in Fluidised Catalytic Cracking (FCC) units to increase the yield of LPG alkenes by conversion of gasoline-range hydrocarbons, forming a key link in the supply chain of these important feedstocks. Improving their yield is therefore a favoured route for meeting the current shortage of propene in the global petrochemicals market. The structure and acidity of the ZSM-5 are known to change over its catalytic lifetime due to steam dealumination of the framework. These changes have been observed to result in significant differences in the interactions between catalyst and substrate between fresh and steamed zeolite. This proposal aims to compare the behaviour of propene and a model gasoline-range alkene (1-octene) when introduced to a simulated industrial ZSM-5 FCC catalyst to those previously observed for a moderately steamed zeolite (RB1810123).
Principal Investigator: Professor David Lennon
Experimenter: Ms Andrea Zachariou
Experimenter: Dr Paul Collier
Experimenter: Dr Alexander Hawkins
Experimenter: Professor Stewart Parker
DOI: 10.5286/ISIS.E.RB1820118
ISIS Experiment Number: RB1820118
Part DOI | Instrument | Public release date | Download Link |
---|---|---|---|
10.5286/ISIS.E.99687776 | TOSCA | 23 November 2021 | Download |
10.5286/ISIS.E.99687823 | TOSCA | 23 November 2021 | Download |
Publisher: STFC ISIS Neutron and Muon Source
Data format: RAW/Nexus
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Data Citation
The recommended format for citing this dataset in a research
publication is as:
[author], [date], [title], [publisher],
[doi]
For Example:
Professor David Lennon et al; (2018): Studies of catalyst-substrate interactions in an industrial ZSM-5 cracking catalyst, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB1820118