ISIS Neutron and Muon Source Data Journal

Study of the exotic quantum magnetic state in paratacamite

Abstract: Since the discovery of spin-liquid behaviors in herbertsmithite ZnCu3(OH)6Cl2, thousands of papers have been published on this subject. However, it remains an open issue about the intrinsic nature of the ground state in herbertsmithite, because ZnCu3(OH)6Cl2 was obtained by substituting Cu2(OH)3Cl [or exprssed as Cu4(OH)6Cl2] and inevitably contained a lot of defects. Previously we found unconventional magnetic transitions and coexistence of order and spin fluctuations in clinoatacamite, Cu2(OH)3Cl [2005 Phys. Rev. Lett. 95 057201], which was the parent compound of herbertsmithite [ZnCu3(OH)6Cl2, which was obtained by substituting Cu with non-magnetic Zn]. Fortunately, now we succeeded in synthesizing single crystals of paratacamite Cu2(OH)3Cl which is a polymorphous structure to clinoatacamite but with high symmetry like herbertsmithite. It is the optimum compound to study with muSR.

Public release date: 22 November 2023

Principal Investigator: Professor Xu-Guang Zheng
Local Contact: Dr Stephen Cottrell
Experimenter: Dr Ichihiro Yamauchi
Local Contact: Dr Adam Berlie
Experimenter: Dr Isao Watanabe
Local Contact: Dr Mark Telling

DOI: 10.5286/ISIS.E.RB1970101-2

Parent DOI: 10.5286/ISIS.E.RB1970101

ISIS Experiment Number: RB1970101

Part Number: 2

Date of Experiment: 16 November 2020

Publisher: STFC ISIS Neutron and Muon Source

Data format: RAW/Nexus
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Data Citation

The recommended format for citing this dataset in a research publication is as:
[author], [date], [title], [publisher], [doi]

For Example:
Professor Xu-Guang Zheng et al; (2020): Study of the exotic quantum magnetic state in paratacamite, STFC ISIS Neutron and Muon Source, https://doi.org/10.5286/ISIS.E.RB1970101-2

Data is released under the CC-BY-4.0 license.